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In this volume we try to review the available literature by two independentapproaches to Nd and Ln-catalyzed diene polymerizations. In the first part ofthe volume, which is entitled “Neodymium-Based Ziegler/Natta Catalysts andtheir Application in Diene Polymerization”, a polymer chemist’s view is givenwith strong emphasis on Nd-based catalyst systems. Also technological andindustrial aspects of Nd-catalyzed diene polymerizations are addressed. In thesecond part of the volume, which is entitled “Rare-Earth Metals and AluminumGetting Close in Ziegler-type Organometallics”, a more organometallic per-spective is given and Ln-based catalyst systems are addressed. By the synopsisof these different perspectives, the reader will comprehend the complexity ofLn-based Ziegler catalyst systems and their application to the polymerizationof dienes.